| Title | Artist | Time | ||
|---|---|---|---|---|
| 1 | The Grimoires | Henry Jackman | 1:16 | |
| 2 | Smurf Village | Henry Jackman | 2:03 | |
| 3 | No Name | Henry Jackman | 3:12 | |
| 4 | Razamel | Henry Jackman | 4:01 | |
| 5 | Neighborhood Watch | Henry Jackman | 1:19 | |
| 6 | Kent's Lair | Henry Jackman | 1:56 | |
| 7 | Smurf's Unite | Henry Jackman | 1:10 | |
| 8 | Land of the Snooterpoots | Henry Jackman | 1:48 | |
| 9 | Mama Poot | Henry Jackman | 1:42 | |
| 10 | Charge of the Smurf Brigade | Henry Jackman | 2:06 | |
| 11 | Echoes of the Past | Henry Jackman | 0:42 | |
| 12 | Storming the Castle | Henry Jackman | 1:35 | |
| 13 | A Valiant Effort | Henry Jackman | 1:59 | |
| 14 | One of Us | Henry Jackman | 1:29 | |
| 15 | The Rise and Fall of Gargamel | Henry Jackman | 1:28 | |
| 16 | The Legend of Ron | Henry Jackman | 2:46 | |
| 17 | Guardianeers | Henry Jackman | 1:29 | |
| 18 | Hostile Takeover | Henry Jackman | 2:04 | |
| 19 | Dreams and Nightmares | Henry Jackman | 1:45 | |
| 20 | Identity Crisis | Henry Jackman | 1:10 | |
| 21 | Long Awaited Epiphany | Henry Jackman | 2:19 | |
| 22 | The Comeuppance | Henry Jackman | 1:45 | |
| 23 | An Unexpected Return | Henry Jackman | 0:56 | |
| 24 | The Wizard Part 1 | Henry Jackman | 4:59 | |
| 25 | The Wizard Part 2 | Henry Jackman | 2:51 |
